This research focuses on optimizing machining parameters and improving surface quality of Al2024/SICp composites crucial for aerospace applications, employing Taguchi design and artificial neural network (ANN) modeling. The optimal parameters identified include a cutting speed of 105 m/min, feed rate of 0.15 mm/rev, and depth of cut of 0.35 mm, achieving minimal surface roughness of 0.9 μm. The findings underscore the potential for enhanced manufacturing practices and component performance in aerospace engineering through systematic experimentation and predictive modeling.